Jack Angel

Papa Smurf (voice)

Fred Armisen

Brainy (voice)

Hank Azaria

Gargamel (voice)

Gary Basaraba

Hefty (voice)

George López

Grouchy (voice)

Melissa Sturm

Smurfette (voice)

Anton Yelchin

Clumsy (voice)

Frank Welker

Azrael (voice)

Kirk Baily

Additional Voices (voice)

Jess Harnell

Additional Voices (voice)

Jeff Fischer

Additional Voices (voice)

Craig Kellman

Additional Voices (voice)